Poster Presentation Australian Society for Microbiology Annual Scientific Meeting 2014

QacA-mediated Multidrug Resistance: Importance of Transmembrane Spanning Region 4   (#228)

Mohsen Chitsaz 1 , Uwe H. Stroeher 1 , Angela Parker 1 , Melissa H. Brown 1
  1. School of Biological Sciences, Flinders University, Adelaide, SA, Australia

The staphylococcal multidrug resistance gene, qacA, confers resistance to an exceptional number of antimicrobial agents, many of which are commonly used as antiseptics and disinfectants. Importantly, the plasmid-borne qacA gene is carried by prevalent clinical isolates of the human pathogen Staphylococcus aureus. The QacA 514-amino acid exporter possesses 14 transmembrane alpha-helices (TMS) and belongs to the major facilitator superfamily (MFS) of transport proteins. It mediates resistance to structurally-unrelated antimicrobials via a proton motive force-dependent mechanism. To gain further insight into this mechanism QacA amino acid residues Ser106 through to Pro139, proposed to be situated within TMS4 and the loops between TMS3:TMS4:TMS5, were subjected to cysteine-scanning mutagenesis. Thirty four residues were individually substituted with cysteine and resulting QacA protein derivatives examined for a number of characteristics including; the ability to efflux the substrate ethidium, solvent accessibility of introduced cysteines as gauged by fluorescein maleimide binding, as well as determination of the resistance profile to a representative set of six antimicrobial compounds. A number of residues were identified, that when substituted, showed a reduced ability to efflux ethidium and/or altered resistance to selected antimicrobials. The majority of these functionally-important residues are highly conserved in the drug/proton antiporter (DHA) family of MFS drug export proteins. Fluorescein maleimide was able to strongly label a number of residues within TMS4 and preincubation with maleimide reduced ethidium efflux for some mutants. Taken together, these results identify a number of residues in the TMS 4 region of QacA essential for the binding and export of cationic antimicrobial compounds and confirm the topology model of QacA predicted by hydropathy analysis.